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“Violence,” came the retort, “is the last refuge of the incompetent.”

Isaac Asimov book Foundation

Variant: Violence is the last refuge of the incompetent.
Source: Part II, The Encyclopedists, section 5; This also appears three times in "Bridle and Saddle" which is titled "The Mayors" within Foundation. It is derived from the famous phrase by Samuel Johnson: "Patriotism is the last refuge of a scoundrel" and from the words of Lady Anne Bellamy in H. Rider Haggard's Dawn, “I do not believe in violence; it is the last resource of fools.” Asimov is usually quoted simply with "Violence is the last refuge of the incompetent."

“It seems to me, Golan, that the advance of civilization is nothing but an exercise in the limiting of privacy.”

Isaac Asimov book Foundation’s Edge

Source: The Foundation series (1951–1993), Foundation’s Edge (1982), Chapter 6 “Earth” section 1, p. 100
Source: Foundation's Edge

“You are the only one responsible for your own wants.”

Isaac Asimov book I, Robot

Source: I, Robot

“A circle has no end.”

Isaac Asimov book Second Foundation

Second Foundation

“Once you get it into your head that somebody is controlling events, you can interpret everything in that light and find no reasonable certainty anywhere.”

Isaac Asimov

Source: The Foundation series (1951–1993), Foundation’s Edge (1982), Chapter 12 “Agent” section 4, p. 226

“The spell of power never quite releases its hold.”

Isaac Asimov

Source: The Foundation series (1951–1993), Second Foundation (1953), Chapter 12 “Lord”

“We abandoned the appearance of power to preserve the essence of it.”

Isaac Asimov

Source: The Foundation series (1951–1993), Foundation’s Edge (1982), Chapter 20 “Conclusion” section 1, p. 408

“[Writing] is an addiction more powerful than alcohol, than nicotine, than crack. I could not conceive of not writing.”

Isaac Asimov

Isaac Asimov's Science Fiction Magazine, April 1990, p.6
General sources

“Outside intelligences, exploring the Solar System with true impartiality, would be quite likely to enter the Sun in their records thus: Star X, spectral class G0, 4 planets plus debris.”

Isaac Asimov

"By Jove!" in View from a Height (1963); often misquoted as "Jupiter plus debris".
General sources

“A robot must protect its own existence as long as such protection does not conflict with the First or Second Laws.”

Isaac Asimov book Runaround

"Runaround" in Astounding Science Fiction (March 1942); later published in I, Robot (1950)
The Three Laws of Robotics (1942)

“To Mankind
And the hope that the war against folly may someday be won, after all.”

Isaac Asimov book The Gods Themselves

Dedication, p. 5; this refers to the quotation of Friedrich Schiller from which Asimov derived the title of this novel: "Against stupidity the gods themselves contend in vain."
The Gods Themselves (1972)

“Courtiers don’t take wagers against the king’s skill. There is the deadly danger of winning.”

Isaac Asimov

Part III, The Mayors, section 3
The Foundation series (1951–1993), Foundation (1951)