“Of the three primary colors, the three binary ones are formed. If you add to one of these the primary tone that is its opposite, it cancels it out. This means that you produce the required half-tone. Therefore, adding black is not adding a half-tone, it is soiling the tone whose true half-tone resides in this opposite me have just described. Hence the green shadows found in red. The heads of the two little peasants. The yellow one had purple shadows; the redder and more sanguine one had green ones.”

—  Paul Signac

Quoted by Maria Buszek, online - note 19 http://mariabuszek.com/mariabuszek/kcai/Expressionism/Readings/SignacDelaNeo.pdf
The notebook where this sentence appears was only published, in facsimile, in 1913 by J. Guiffrey. Signac therefore must have consulted it at the Conde Museum, in Chantilly. This Moroccan travel document was bought at the Delacroix sale by the painter Dauzats for the Duc of Aumale.
From Delacroix to Neo-Impressionism, 1899

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Paul Signac 9
French painter 1863–1935

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Quote from Maria Buszek, online - note 22 http://mariabuszek.com/mariabuszek/kcai/Expressionism/Readings/SignacDelaNeo.pdf
Seurat's quote from: Jules Christophe, Seurat, in 'Les Hommes d'aujourd'hui', no. 368, March-April 1890
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